巻号一覧
18 巻, 9 号
選択された号の論文の36件中1～36を表示しています
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浅井 満子1970 年 18 巻 9 号 p. 1699-1705
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーA molecular formula, C38H38O11, has been given for pillaromycin A. Acid hydrolysis of pillaromycin A afforded an aglycone, pillaromycinone, C20H18O7 and a new sugar, pillarose, C8H12O5. From the results of spectrometrical and chemical studies on pillaromycinone and its derivatives the presence of the following functional groups was elucidated in pillaromycinone ; two sec-hydroxyls, a tert-hydroxyl, two phenolic hydroxyls, a chelated carbonyl and an acetyl conjugated with α, β-unsaturated double bond.抄録全体を表示PDF形式でダウンロード (809K) -
浅井 満子1970 年 18 巻 9 号 p. 1706-1712
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe structure of pillaromycinone (II) was elucidated. The ultraviolet (UV) spectrum of PMN tetraacetate (VI) was similar to that of 1, 2, 3, 4-tetrahydro-1-oxophenanthrene. On oxidative degradation pillaromycinone dimethyl ether (IX) gave 3-methoxy-1, 2, 4, 5-benzenetetracarboxylic acid (X) and 3-methoxyphthalic acid (XI). Zinc dust distillation of II gave anthracene and naphthacene. The UV spectrum of II resembles to that of anhydrodemethyltetracycline. From the chemical and spectrometric data the structure of β-substance (IV) was suggested to be 1, 2, 3, 4, 4a, 5, 12, 12a-octahydro-12-oxo-4, 10, 11, 12a-tetrahydroxynaphthacene. The nuclear magnetic resonance (NMR) and the spin decouplings of isopropylidene PMN (XVI) and PMN (II) gave the structure (3(S), 4(R), 4a(R), 12a(R)) 2-acetyl-3, 4, 4a, 5, 12, 12a-hexahydro-12-oxo-3, 4, 10, 11, 12a-pentahydroxynaphthacene to PMN (II).抄録全体を表示PDF形式でダウンロード (722K) -
浅井 満子1970 年 18 巻 9 号 p. 1713-1719
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPillarose (I), C8H12O5, gives positive Fehling's and iodoform reactions. Absorption of an isolated carbonyl is observed in the infrared and ultraviolet region. I formed methyl pillarosides (VIIa, b) and mono-, diacetylpillaroses, and reacted with sodium borohydride to yield methyl dihydropillarosides (Xa, b). I consumed 2 moles of periodate. Periodate oxidation of I in acidic solution gave acetaldehyde, formic acid (and formaldehyde), succinaldehydic acid and carbon dioxide. From these degradation schemes and physico chemical properties of the above derivatives the structure, 2, 3, 6-trideoxy-2-glycoloylhexopyranos-4-ulose, was given to pillarose (I).抄録全体を表示PDF形式でダウンロード (724K) -
浅井 満子, 水田 栄治, 水野 公明, 三宅 彰, 立岡 末雄1970 年 18 巻 9 号 p. 1720-1723
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe structure of pillaromycin A (I, PMA), C28H28O11, is elucidated as I. In PMA (I) 12a hydroxyl of pillaromycinone (II, PMN), C20H18O7, is linked glycosidicaly to the 1'-anomeric hydroxyl of pillarose (III), C8H12O5.抄録全体を表示PDF形式でダウンロード (406K) -
神谷 和秀, 浅井 満子, 西川 正夫, 水野 公明, 富家 勇次郎, 新田 勇1970 年 18 巻 9 号 p. 1724-1730
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーIn order to confirm the chemical and stereochemical structure of pillaronone, a derivative of the aglycone obtained from pillaromycin A, an X-ray analysis of its monobromoacetate has been carried out. Pillaronone monobromoacetate crystallizes in the orthorhombic system, space group P212121-D42, with four molecules of C22H19O6Br in a unit cell. Application of a three-dimensional Patterson superposition method facilitated the elucidation of the structure which is given in formula (I). The final R-value was 0.133. The absolute configuration was determined using the anomalous dispersion of the bromine atom. The molecular structure in the crystal was also discussed.抄録全体を表示PDF形式でダウンロード (812K) -
斎藤 勲, 菊川 靖雄, 山田 俊一1970 年 18 巻 9 号 p. 1731-1736
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーTertiary amides of five amino acids and their derivatives were reduced with sodium borohydride in refluxing pyridine to the corresponding diamines in moderate yields. Effects of substituents at the α-position on α-substituted N, N-dimethylhydrocinnamamide were examined.抄録全体を表示PDF形式でダウンロード (745K) -
南原 利夫, 高橋 洋井, 上川 やよい1970 年 18 巻 9 号 p. 1737-1741
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーFor the studies on metabolic fate of 3-deoxydehydroepiandrosterone in man, 5-dehydro- and 5β-androstanes having oxygen functions at both C-2 and C-17, the possible metabolites, have been synthesized as shown in Chart 1.抄録全体を表示PDF形式でダウンロード (658K) -
浜名 政和, 熊懐 稜丸1970 年 18 巻 9 号 p. 1742-1750
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーIndole (II) was found to react as an aromatic analog of enamine with acyl-adducts of quinoline 1-oxide (I) and ethyl nicotinate 1-oxide (VI) under refluxing condition in chloroform, and 3-(2-quinolyl) indole (III) and ethyl 6-(3-indolyl) nicotinate (VII) were obtained, respectively, but no reaction occured with pyridine 1-oxide. Benzoyl chloride was most effective as an acylating agent. 1-Methylindole (VIII) underwent similar reactions. The reaction with I gave 1-methyl derivative of III (IX) as well as 4-quinolyl compound (X). From the reaction with 2-chloroquinoline 1-oxide (XI), 1-methyl-3-(2-chloro-4-quinolyl) indole (XIII) and 1-benzoyloxy-2-hydroxy-4-(1-methyl-3-indolyl)-1, 4-dihydroquinoline (XIV) were produced, the isolation of XIV being significant from the mechanistic view point. 4-Chloroquinoline 1-oxide and VIII afforded 2-quinolyl compound (XVI). Further 2-phenylindole was shown to react with I under similar conditions, but skatole resisted the reaction.抄録全体を表示PDF形式でダウンロード (953K) -
金子 秀彦, 大和 讓, 黒川 美貴雄1970 年 18 巻 9 号 p. 1751-1758
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーAddition of ethyl mercaptan to 6-dehydro-17α-methyltestosterone (I) in the presence of the organic bases afforded two oxidative addition products together with the corresponding 7α-ethylthio derivative (II) in minor yields. Both of them were formulated as 6α-hydroxy-7β-ethylthio- and 6β-hydroxy-7α-ethylthio-17α-methyltestosterone (III and IV) by chemical evidences and the spectral data. Under similar condition, androsta-4, 6-diene-3, 17-dione (XII) gave an unexpected compound, 4-ethylthio-7β-hydroxyandrost-4-en-3-one (XXIII) accompanied with 7α-ethylthio (XIII), 6α-hydroxy-7β-ethylthio (XIV) and 6β-hydroxy-7α-ethylthio derivative (XV).抄録全体を表示PDF形式でダウンロード (954K) -
佐々木 喜男, 鈴木 美代子1970 年 18 巻 9 号 p. 1759-1773
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe Electronic Indices : π-Electron charge density ρ, Fr, Sr(E), Sr(R) and Sr(N) : were obtained for monosubstituted-benzene, 1-substituted-3, 4-dimethoxybenzene, 2-substitutednaphthalene and 2-substituted-6-methoxy-naphthalene derivatives, and the following results were obtained. 1. The ρ values are linearly related with the substituent constant σπ. 2. Fr, Sr(E), Sr(R) and Sr(N) are linearly related with the substituent constant σπ when the substituent groups are electron releasing, but not when they are electron attracting. 3. The electronic indices of polysubstituted benzene derivatives expressed by the simple sum of the excess value Δ with reference to benzene are comparable with calculated values.抄録全体を表示PDF形式でダウンロード (962K) -
佐々木 喜男, 鈴木 美代子1970 年 18 巻 9 号 p. 1774-1787
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe electronic indices : π-electron charge density ρ, Fr, Sr(E), Sr(R) and Sr(N) : were obtained for 3-and 4-substituted pyridine, 6-substituted quinoline and 6-substituted quinoxaline derivatives, and the following results were obtained. 1. The ρ values are linearly related to the substituent constant σπ. 2. Fr, Sr(E), Sr(R) and Sr(N) are linearly related with σπ for electron releasing substituent group sites, but this linear relation does not hold for electron attracting substituent group sites. 3. The reliability of the simple sum rule of molecular electronic indices was confirmed.抄録全体を表示PDF形式でダウンロード (840K) -
松尾 寿之, 川添 豊, 佐藤 要, 大西 柾子, 辰野 高司1970 年 18 巻 9 号 p. 1788-1793
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (672K) -
佐藤 要, 辰野 高司, 松尾 寿之1970 年 18 巻 9 号 p. 1794-1798
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーKinetical study was carried out in the base-catalyzed racemization reaction of N-benzoyl anilide derivatives of six neutral amino acids, such as alanine, α-aminobutyric acid, valine, leucine, phenylalanine and phenylglycine. From the comparison of rate-constants thus obtained, it was concluded that the susceptibility of amino acids tested to the racemization may be expressed in thrm of acidity of α-proton related to the electronnegativity of alkyl-, aralkyl- and aryl-side chains at α-carbon.抄録全体を表示PDF形式でダウンロード (575K) -
宮野 和子, 田口 胤三1970 年 18 巻 9 号 p. 1799-1805
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPhenylmagnesium bromide reacted with 2-cyclohexylidenecyclohexanone (I) affording 2-(1-phenylcyclohexyl) cyclohexanone (II) in main, via 1, 4-addition. Besides, it accompanied 6-(1-phenylcyclohexyl)-6-oxo-hexanoic acid (III) as by-product, even though the reaction was carried out in a stream of nitrogen, using purified ether as a solvent. It was found that (a) III itself did not exist just after the Grignard reaction and appeared after heating of the reaction mixture at 70-80° ; (b) the ketone II, even in the enol form, did not produce a substance which convert into III by the absorption of oxygen. This suggested that the III-precursor, presumably a peroxide, was produced in the course of the Grignard reaction, thereafter transformed to III. Reactions for the identification of III and the Grignard reaction of other α, β-unsaturated ketones were persued.抄録全体を表示PDF形式でダウンロード (829K) -
宮野 和子, 田口 胤三1970 年 18 巻 9 号 p. 1806-1814
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーA novel intramolecular cyclization reaction was found in the reaction of 2 (1'-phenyl)-cyclohexylcyclohexanone oxime (I-oxime) with aromatic Grignard reagent, either phenyl- or p-tolylmagnesium bromide, which worked as a catalyst. The reaction required at least 3 equivalent moles of Grignard reagent. The structure of the cyclization product (II) was established as spiro [bicyclo [3.3.1]-3, 4-benzononan-9-one-2, 1'-cyclohexane]. The structural feature of oximes which suffer the cyclization reaction was preliminary discussed.抄録全体を表示PDF形式でダウンロード (871K) -
岡本 敏彦, 磯谷 遥, 小泉 徹1970 年 18 巻 9 号 p. 1815-1821
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe quantitative estimation methods were established for Me-IAA, IAN, PAM, IAM, IAA, and PHCA by gas chromatography and colorimetry.抄録全体を表示PDF形式でダウンロード (664K) -
浜名 政和, 熊懐 稜丸1970 年 18 巻 9 号 p. 1822-1830
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリー1-Methyloxindole (II) reacted as an active methylene compound with acyl-adducts of quinoline 1-oxides (I, IX and VIII), forming 1-methyl-3-(2- or 4-quinolyl)oxindoles (III, XV or XI). The reaction with I in the presence of acetic anhydride or benzoyl chloride further proceeded and gave bis-quinolyl compound (IV) besides mono-quinolyl one (III). The order of effectiveness of acylating agents was acetic anhydride>benzoyl chloride>tosyl chloride. Pyridine 1-oxide (XVII) itself was also able to react with II in hot acetic anhydride to give four kinds of products, 2-pyridyl- (XX), bis-2-pyridyl- (XIX), 4-pyridyl-product (XXI) and acetate of XXI (XVIII). The reaction of oxindole (XXVI) with I progressed similarly and 3-(2-quinolyl)-oxindole (XXVII) was obtained.抄録全体を表示PDF形式でダウンロード (1023K) -
高橋 幸太郎, 高荷 昌子1970 年 18 巻 9 号 p. 1831-1840
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリー1) The structures of two pyrolysis products of methyldihydrousnic acid (I) were established to be II and III, respectively. 2) The mechanism of the formation of II and III from I were discussed. 3) The mass spectra of V and isoanhydromethyldihydrousnic acid monoacetate, and X and anhydromethyldihydrousnic acid monoacetate were studied.抄録全体を表示PDF形式でダウンロード (914K) -
石渡 三郎, 板倉 啓壹1970 年 18 巻 9 号 p. 1841-1845
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリー8-Amino-1, 2, 3, 4-tetrahydro-7-methoxy-1-(4-methoxybenzyl)-2-methyl-6-isoquinolinol (IIa) was synthesized and the Pschorr reaction of this compound under alkaline conditions gave dl-homolinearisine, which could not be synthesized by the phenolic oxidative coupling method. Infrared and nuclear magnetic resonance spectra of the synthesized sample were superimposable with those of the natural product.抄録全体を表示PDF形式でダウンロード (586K) -
石渡 三郎, 板倉 啓壹1970 年 18 巻 9 号 p. 1846-1849
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe Mannich reaction of tetrahydroisoquinolines (IVa, b) with 36% formalin in acetic acid gave respectively protoberberines (Va, b) and each compounds were converted to tetramethoxyprotoberberines (Ic, d). Ic was identified by the infrared and nuclear magnetic resonance spectral comparisons with caseadine methyl ether derived from natural caseamine or caseadine. Hydrochloric acid catalyzed condensation of 7, 8-disubstituted tetrahydroisoquinoline (VIII) with 36% formalin gave the same compound (Ic).抄録全体を表示PDF形式でダウンロード (533K) -
石渡 三郎, 藤井 起二, 宮司 進之, 佐藤 吉之, 板倉 啓壹1970 年 18 巻 9 号 p. 1850-1855
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe Bischler-Napieralski reaction of the phenethylamides (VIIa and VIIb) gave respectively the 6-ethoxycarbamido-3, 4-dihydroisoquinolines, formed by the cyclization at the position para to the ethoxycarbamido group, and both 3, 4-dihydroisoquinolines were converted to the 6-aminoisoquinolines (Xa and Xb). Each 7, 8-disubstituted isoquinolines (XIIa and XIIb), prepared by deamination reaction of Xa and Xb, were submitted to the Ullmann reaction to give respectively 6-methoxy-1-methyl-1, 2, 3, 12, 12a-pentahydrobenzoxepino [2, 3, 4-i, j] isoquinoline (XIII) and dl-cularine (Ia).抄録全体を表示PDF形式でダウンロード (689K) -
井上 博之, 上田 伸一, 中村 有伸1970 年 18 巻 9 号 p. 1856-1865
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーAus Swertia japonica MAKINO wurden neben Swertiamarin (I) folgende vier Glucoside isoliert, die auch bitter schmecken und zu den Secoiridoid-Glucosiden zu zahlen sind : Amarogentin, Amaroswerin, Gentiopicrosid (II) und Sweroid (III). Weiter wurden die Absolutstrukturen des Swertiamarins (I), des Gentiopicrosids (II) und des Sweroids (III) klargestellt.抄録全体を表示PDF形式でダウンロード (1164K) -
山口 良二, 鈴木 はな, 平島 弘子1970 年 18 巻 9 号 p. 1866-1871
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーUse of o-chlorophenol instead of salicylate improved the sensitivity of salicylate-2, 6-dichloroisocyanurate method for the determination of ammonia. By the use of 2, 6-dichloroisocyanurate, the stored oxidant solution became more stable than sodium hypochlorite, which had been commonly used up to now. The presence of a micro-amount of sodium nitroprusside was necessary. Apparent molar extinction coefficient on the basis of nitrogen atom and coefficient of variation at 15.15μg/ml ammonium sulfate were 3.14×104 and 1.83%, respectively. Absorbance of the reagent blank at 665 mμ was as low as 0.058±0.005.抄録全体を表示PDF形式でダウンロード (589K) -
磯谷 遥, 菰田 泰夫, 岡本 敏彦1970 年 18 巻 9 号 p. 1872-1879
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーA pea inhibitor was isolated as natural free acid and as its methyl ester from the garden peas (Pisum sativum L.) and they were identified with (+)-abscisic acid (Ia) and its methyl ester (Ib), respectively. On the other hand, sayanedine, mp 165-166°, C17H14O5, which is a new isoflavone and which had kinetin-like activity in the tabacco pith callus bioassay, was also isolated from the same plant, and its chemical structure was confirmed to be 4'-hydroxy-7, 3'-dimethoxyisoflavone (VI) on the basis of spectral and synthetic evidences.抄録全体を表示PDF形式でダウンロード (935K) -
石井 永, 安井 凡平, 西野 隆一, 原山 尚, 犬伏 康夫1970 年 18 巻 9 号 p. 1880-1888
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーStructures of two Lycopodium alkaloids, serratinidine (I) from Lycopodium serratum THUNB. var. serratum f. serratum and fawcettidine (XIX) from Lycopodium fawcettii LYLOYD et UNDERWOOD, were examined. In the previous papers, the authors suggested the biogenesis of serratinine and in connection of this, the skeletal structure ((B) in Chart 1) for serratinidine was selected as a working hypothesis. The validity of this assumption was shown by chemical correlation of serratinine ((C), R=OH, in Chart 1) of established structure with serratinidine through the route shown in Chart 2. On the other hand, fawcettidine was first isolated by Burnell from a Jamaican Lycopodium plant but since then there has been no report on the structure. From physical and spectral properties of this alkaloid appeared in the literature, the authors postulated the same skeletal structure for fawcettidine as that of serratinidine. Then, this assumption was proved by chemical conversion of serratinine into fawcettidine along the schemes shown in Chart 5. The present study reveals a new structural type of Lycopodium alkaloid.抄録全体を表示PDF形式でダウンロード (1098K) -
井上 博之, 吉田 隆志, 中村 有伸, 飛田 修作1970 年 18 巻 9 号 p. 1889-1899
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーDurch die Uberfuhrung des in der Absolutstruktur abgeklarten Asperulosids (IV) und des Swerosids (III) zu 9-Epidihydroswerosid-tetraacetat ist die chemische Korrelation der beiden Naturstoffe festgestellt. Dabei wurde weiter die Stereochemie der Aglucone von Dihydroswerosid (XXVIII), α-Tetrahydrogentiopicrosid (XXV) und 9-Epidihydroswerosid sowie die der aus diesen Agluconen abgeleiteten Dilactone diskutiert.抄録全体を表示PDF形式でダウンロード (1199K) -
高畠 英伍, 児玉 龍平, 田中 良明, 堂森 廉三, 立沢 晴男, 内藤 武男1970 年 18 巻 9 号 p. 1900-1907
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーThe metabolic fate of 1-(4-methoxy-6-methyl-2-pyrimidinyl)-3-methyl-5-methoxy-pyrazole (mepirizole, DA-398) was investigated in rat and rabbit. Four metabolites were isolated as crystals from the urine of medicated rats and identified as 1-(4-methoxy-5-hydroxy-6-methyl-2-pyrimidinyl)-3-methyl-5-methoxypyrazole (UNM-1), 1-(4-methoxy-6-methyl-2-pyrimidinyl)-3-hydroxymethyl-5-methoxypyrazole (UNM-2), 1-(4-methoxy-6-methyl-2-pyrimidinyl)-5-methoxypyrazole-3-carboxylic acid (UAM-1) and 1-(4-methoxy-6-methyl-2-pyrimidinyl)-3-methyl-4-hydroxy-5-methoxypyrazole sulfate (URM-1). From the rabbit urine, UAM, UNM-2, UNM-4 (1-(4-methoxy-6-hydroxymethyl-2-pyrimidinyl)-3-methyl-5-methoxypyrazole) were isolated and the excretion of UNM-1, UNM-3 (2-hydroxy-4-methoxy-6-methylpyrimidine) and UNM-5 (1-(4-methoxy-6-methyl-2-pyrimidinyl)-3-methyl-4-hydroxy-5-methoxypyrazole) were identified on thin-layer chromatogram. The major metabolite was UAM-1 both in rat and in rabbit.抄録全体を表示PDF形式でダウンロード (838K) -
堂森 廉三, 吉村 龍一, 北原 [しん]一, 田中 良明, 内藤 武男1970 年 18 巻 9 号 p. 1908-1914
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーAll the metabolites (UAM-1, UNM-1, UNM-2, UNM-4, and URM-1), which were isolated from the urine of rats and rabbits administered 1-(4-methoxy-6-methyl-2-pyrimidinyl)-3-methyl-5-methoxypyrazole (mepirizole, DA-398) were synthesized and their structures were established by direct comparison with the synthetic samples.抄録全体を表示PDF形式でダウンロード (821K) -
金沢 治男, 小原 晃, 吉岡 政七1970 年 18 巻 9 号 p. 1915-1917
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (424K) -
金沢 治男, 石光 進, 清水 康紘, 田中 茂, 玉井 敏夫, 小原 晃, 吉岡 政七1970 年 18 巻 9 号 p. 1918-1920
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーIn the previous paper, it was reported that the cyanide-activated papain is apparently inhibited by active methylene group and active imide group in barbituric acid. The active methylene group in barbituric acid is derived from malonic acid. Morgan and Friedmann have been shown that maleic acid and SH-compounds interact with the formation of stable addition compounds. They have applied this reaction to the study of some SH-enzyme reaction. The present research has been planed to clarify relation between activity of papain and influence of the dibasic acids.抄録全体を表示PDF形式でダウンロード (408K) -
喜谷 喜徳, 加藤 征将, 小池 久1970 年 18 巻 9 号 p. 1921-1924
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (466K) -
西垣 貞男, 千賀 慶太郎, 米田 文郎1970 年 18 巻 9 号 p. 1925-1926
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (369K) -
高畠 英伍, 児玉 龍平1970 年 18 巻 9 号 p. 1927-1929
発行日: 1970/09/25
公開日: 2008/03/31
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植田 寛, 吉岡 一郎1970 年 18 巻 9 号 p. 1931-1933
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (431K) -
宮崎 元一, 金子 春一1970 年 18 巻 9 号 p. 1933-1934
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (371K) -
中嶋 暉躬, 遠藤 仁, 酒井 文徳, 田村 善蔵1970 年 18 巻 9 号 p. 1935
発行日: 1970/09/25
公開日: 2008/03/31
ジャーナル フリーPDF形式でダウンロード (270K)
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